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H.I.V.E.: Higher Institute of Villainous Education by Mark Walden: "Swept away to a hidden academy for training budding evil geniuses, Otto, a brilliant orphan, Wing, a sensitive warrior, Laura, a shy computer specialist, and Shelby, an infamous jewel thief, plot to beat the odds and escape the prison known as H.I.V.E." (Book Description)
If you like H.I.V.E.: Higher Institute of Villainous Education, you may also like these titles:
Artemis Fowl by Eoin Colfer.
Twelve-year-old Artemis Fowl is the most ingenious criminal mastermind in history. With two trusty sidekicks in tow, he hatches a cunning plot to divest the fairyfolk of their pot of gold. Of course, he isn't foolish enough to believe in all that "gold at the end of the rainbow" nonsense. Rather, he knows that the only way to separate the little people from their stash is to kidnap one of them and wait for the ransom to arrive. You will love this evil-doer! Read all of the books in this series!
The Girl Who Could Fly by Victoria Forester.
The perfect companion to H.I.V.E., except a little less evil. This is one of my favorites! When homeschooled farm girl Piper McCloud reveals her ability to fly, she is quickly taken to a secret government facility to be trained with other exceptional children, but she soon realizes that something is very wrong and begins working with brilliant and wealthy Conrad to escape.